Keywords LR and smart folder Mac

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To build on WobertC's reply:

1. Finder can't see LR catalog metadata unless you've written it back to the photo files. Make sure you've selected all the photos and done Metadata > Save Metadata To File, or better, check the option Catalog Settings > Metadata > Automatically Write Changes Into XMP. 

2. Finder doesn't know that .xmp sidecars, which store the metadata for raws, are associated with their corresponding raws. It will search the sidecars' text contents, though it doesn't understand the industry metadata standards and how keywords get stored in particular fields within the sidecars.  So if you want to search both non-raws (JPEGs, TIFFs, PSDs) and raws' sidecars for a keyword, you'd have to do something like this:

That second criterion, "Contents contains zzyyxx", will match any kind of file containing "zzyyxx", so if necessary, you could further refine the criteria to restrict it just to .xmp sidecars.

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Could the files that do not display be 'raw'?

(In Windows) Saving Keywords to raw files [Ctrl+S] in Lr-Classic creates a separate XMP file with this metadata.

In Windows File Explorer the raw file does not show a 'Tag' (Keyword) in File Properties.

If this were the same in a Mac, the Smart Folder may not detect any Keywords in raw files.

2. What Filters are applied?

Full screenshot would help

Smart Folder? Do you mean Smart Collection?

1. For the Smart Collection, list your rules.